Isostructural metal-insulator transition driven by dimensional-crossover in <mml:math xmlns:mml="http://www.w3.org/1998/Math/MathML"><mml:msub><mml:mi>SrIrO</mml:mi><mml:mn>3</mml:mn></mml:msub></mml:math> heterostructures

نویسندگان

چکیده

Dimensionality reduction induced metal-insulator transitions in oxide heterostructures are usually coupled with structural and magnetic phase transitions, which complicate the interpretation of underlying physics. Therefore, achieving isostructural MIT is great importance for fundamental physics even more applications. Here, we report an transition driven by dimensional-crossover spin-orbital SrIrO3 films. By using in-situ pulsed laser deposition angle-resolved photoemission spectroscopy, synthesized investigated electronic structure ultrathin films atomic-layer precision. Through inserting orthorhombic CaTiO3 buffer layers, demonstrate that crystal remains bulk-like similar oxygen octahedra rotation tilting when approaching limit. We observe a occurs Intriguingly, find bandwidth Jeff=3/2 states reduces lowering dimensionality drives transition. Our results establish controlled thin

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ژورنال

عنوان ژورنال: Physical Review Materials

سال: 2022

ISSN: ['2476-0455', '2475-9953']

DOI: https://doi.org/10.1103/physrevmaterials.6.034404